Methoxy-substituted 9-aminomethyl-9,10-dihydroanthracene (AMDA) derivatives exhibit differential binding affinities at the 5-HT(2A) receptor. Bioorg Med Chem Lett 2008 Oct 01;18(19):5268-71
Date
09/09/2008Pubmed ID
18774714Pubmed Central ID
PMC3082371DOI
10.1016/j.bmcl.2008.08.059Scopus ID
2-s2.0-52249112061 (requires institutional sign-in at Scopus site) 10 CitationsAbstract
The effects of methoxy-substitution at the 1-, 2-, 3-, and 4-positions of 9-aminomethyl-9,10-dihydroanthracene (AMDA) on h5-HT(2A) receptor affinity were determined. Racemic mixtures of these compounds were found to show the following affinity trend: 3-MeO > 4-MeO > 1-MeO approximately 2-MeO. Comparison of the effects of these substitutions, with the aid of computational molecular modeling techniques, suggest that the various positional and stereochemical isomers of the methoxy-substituted AMDA compounds interact differently with the h5-HT(2A) receptor. It is predicted that for the compounds with higher affinities, the methoxy oxygen atom is able to interact with hydrogen bond-donating sidechains within alternative h5-HT(2A) receptor binding sites, whereas the lower-affinity isomers lack this ability.
Author List
Dewkar GK, Peddi S, Mosier PD, Roth BL, Westkaemper RBAuthor
Philip Mosier PhD Assistant Professor in the School of Pharmacy Administration department at Medical College of WisconsinMESH terms used to index this publication - Major topics in bold
AnthracenesCombinatorial Chemistry Techniques
Humans
Models, Molecular
Molecular Structure
Receptor, Serotonin, 5-HT2A
Structure-Activity Relationship